It sounds like you want to return the affinity to the default (keep in mind, this isn't necessarily the same as all processors, the default is is 2^n -1, where n is the number of processors, see the documentation).
To return to the default, simply store the default in a variable and then reassign it.
void Main()
{
Process p = Process.GetProcessById(12008);
var originalAffinity = p.ProcessorAffinity;
Console.WriteLine("Original affinity: " + originalAffinity);
p.ProcessorAffinity = (IntPtr)0x0001;
Console.WriteLine("Current affinity: " + p.ProcessorAffinity);
p.ProcessorAffinity = originalAffinity;
Console.WriteLine("Final affinity: " + p.ProcessorAffinity);
}
Results on my machine:
Original affinity: 255
Current affinity: 1
Final affinity: 255