The duration in the fields there is just a kind of summary. You need to extend the time each single picture is displayed. Do that by manipulating the box found here:
/moov/trak/mdia/minf/stbl/stts
It is the time to sample atom/box. To learn about the content and structure of this atom/box you can safely use the Quicktime File Format Specification if you don't have an ISO/EIC 14496-12 at hand.
To increase or decrease the speed of the video you may multiply every sample duration (most cases just a single one) by a factor.
NOTE: H264 video also has the ctts box in some cases (if B-frames are used). You will need to modify the times there, too.