What does it mean? I can't find any documentation anywhere.
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Have you tried to use Optimize-Volume against VMStorage virtual disk? I also was not able to find description for all possible HealthStatus values in general and for Suboptimal in particular. If no parameters specified Optimize-Volume will perform default action based on disk type:
- HDD, Fixed VHD, Storage Space -Analyze -Defrag.
- Tiered Storage Space -TierOptimize.
- SSD with TRIM support -Retrim.
- Storage Space (Thinly provisioned), SAN Virtual Disk (Thinly provisioned), Dynamic VHD, Differencing VHD -Analyze -SlabConsolidate -Retrim.
- SSD without TRIM support, Removable FAT, Unknown - No operation.
You may also want to look at this TechNet Forums thread which mentions the same status.

Mikhail
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I have not managed to find an exact description of the operational status section also. But I would recommend to check your physical drives participating in that logical disk since it seems like an individual drive failure. I just made some analogies about logical disks on a hardware RAID which actually guided me to this.

batistuta09
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1Yea we had a failure. Optimize-Volume after it fixed the problem. – hex Nov 01 '16 at 16:05
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The following PowerShell command helped me:
Get-StoragePool -FriendlyName "s2d*" | Optimize-StoragePool

chicks
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